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These results suggest how important the role of the hydrophobic effect is on the catalytic activity of the reaction.
Although challenging, the possibility to perform aqueous metatheses has become an attractive alternative, not only because water is a more sustainable medium, but also to exploit biocompatible conditions.
This review focuses on the progress made in aqueous olefin metatheses and their applications in chemical biology.
Keywords: Olefin metathesis represents a versatile synthetic tool for the construction of carbon–carbon bonds [1-9].
Since its first report in 1956, a Ti(II)-catalyzed polymerization of norbornene , metathesis rapidly attracted interest among organic chemists and has been used in different research fields spanning polymer chemistry [11,12] to drug discovery [13-15].
In this specific case, the formation of the metal hydride complex is believed to occur during the work-up with methanol.